| Season | Airdate | Title | Usage | Note |
|---|
| 1 | 1981‑09‑12 (1) | The Astrosmurf | To destroy. | |
| 1 | 1981‑09‑12 (2) | Jokey’s Medicine | To eat. | |
| 1 | 1981‑09‑12 (3) | Vanity Fair | To eat. | |
| 1 | 1981‑09‑19 (1) | St. Smurf And The Dragon | To destroy. | |
| 1 | 1981‑09‑19 (2) | Magical Meanie | None given. | |
| 1 | 1981‑09‑19 (3) | Sorcerer Smurf | To eat. | |
| 1 | 1981‑09‑26 (1) | Bewitched, Bothered, and Besmurfed | To eat. | |
| 1 | 1981‑09‑26 (2) | King Smurf | Does not appear. | |
| 1 | 1981‑09‑26 (3) | The Smurfs And The Howlibird | Does not appear. | |
| 1 | 1981‑10‑03 (1) | Soup A La Smurf | To eat. | |
| 1 | 1981‑10‑03 (2) | All That Glitters Isn’t Smurf | To make gold. | |
| 1 | 1981‑10‑03 (3) | Dreamy’s Nightmare | To eat. | |
| 1 | 1981‑10‑10 (1) | Romeo And Smurfette | To eat. | |
| 1 | 1981‑10‑10 (2) | The Magic Egg | To eat. | |
| 1 | 1981‑10‑10 (3) | Smurphony In ‘C’ | To destroy. | |
| 1 | 1981‑10‑17 (1) | Sideshow Smurfs | None given. | |
| 1 | 1981‑10‑17 (2) | Supersmurf | Does not appear. | |
| 1 | 1981‑10‑17 (3) | Paradise Smurfed | Does not appear. | |
| 1 | 1981‑10‑24 (1) | Sir Hefty | Does not appear. | |
| 1 | 1981‑10‑24 (2) | The Baby Smurf | None given. | Gargamel’s initial purpose is not given, as a fall-back plan he attempts to destroy the smurfs. |
| 1 | 1981‑10‑24 (3) | The Fake Smurf | Does not appear. | |
| 1 | 1981‑10‑31 (1) | Painter And Poet | To eat. | |
| 1 | 1981‑10‑31 (2) | Haunted Smurf | Does not appear. | |
| 1 | 1981‑10‑31 (3) | The Purple Smurfs | Does not appear. | |
| 1 | 1981‑11‑07 (1) | The Fountain Of Smurf | To eat. | |
| 1 | 1981‑11‑07 (2) | The Magnifying Mixture | None given. | |
| 1 | 1981‑11‑07 (3) | Foul Weather Smurf | Does not appear. | |
| 1 | 1981‑11‑14 (1) | The Hundredth Smurf | Does not appear. | |
| 1 | 1981‑11‑14 (2) | The Abominable Snowbeast | Does not appear. | |
| 1 | 1981‑11‑14 (3) | Gargamel, The Generous | To get diamonds. | Gargamel first uses the smurfs to get diamonds, then he tries to destroy the smurfs. |
| 1 | 1981‑11‑21 (1) | The Smurfette | To eat. | |
| 1 | 1981‑11‑21 (2) | Now You Smurf ’Em, Now You Don’t | Does not appear. | |
| 1 | 1981‑11‑21 (3) | Spelunking Smurfs | To eat. | |
| 1 | 1981‑11‑28 (1) | The Smurfs’ Apprentice | To use as test subjects. | Usage revealed in comic book. |
| 1 | 1981‑11‑28 (2) | Smurf-Colored Glasses | None given. | |
| 1 | 1981‑11‑28 (3) | The Clockwork Smurf | Does not appear. | |
| 1 | 1981‑12‑05 (1) | Fuzzle Trouble | To eat. | |
| 1 | 1981‑12‑05 (2) | Smurfette’s Dancing Shoes | Does not appear. | |
| 1 | 1981‑12‑05 (3) | The Smurfs And The Money Tree | To destroy. | |
| 1 | 1982‑04‑08 (1) | The Smurf Springtime Special | To make gold. | Some inconsistencies in whether he would use the smurfs to turn lead into gold, or turn the smurfs into gold. |
| 2 | 1982‑09‑18 (1) | The Smurf Who Couldn’t Say No | Does not appear. | |
| 2 | 1982‑09‑18 (2) | The Adventures Of Robin Smurf | Does not appear. | |
| 2 | 1982‑09‑18 (3) | The Cursed Country | Does not appear. | |
| 2 | 1982‑09‑25 (1) | S-Shivering S-Smurfs | To eat. | |
| 2 | 1982‑09‑25 (2) | Sister Smurf | Does not appear. | |
| 2 | 1982‑09‑25 (3) | The Black Hellebore | Does not appear. | |
| 2 | 1982‑09‑25 (4) | Revenge Of The Smurfs | Does not appear. | |
| 2 | 1982‑10‑02 (1) | The Three Smurfketeers | Does not appear. | |
| 2 | 1982‑10‑02 (2) | Heavenly Smurfs | None given. | |
| 2 | 1982‑10‑02 (3) | It Came From Outer Space | Does not appear. | |
| 2 | 1982‑10‑02 (4) | The Sorcery Of Maltrochu | Does not appear. | |
| 2 | 1982‑10‑09 (1) | Squeaky | Does not appear. | |
| 2 | 1982‑10‑09 (2) | The Kaplowey Scroll | To destroy. | |
| 2 | 1982‑10‑09 (3) | The Goblin of Boulder Wood | Does not appear. | |
| 2 | 1982‑10‑09 (4) | Gormandizing Greedy | To eat. | |
| 2 | 1982‑10‑09 (5) | Waste Not, Smurf Not | Does not appear. | |
| 2 | 1982‑10‑16 (1) | Johan’s Army | Does not appear. | |
| 2 | 1982‑10‑16 (2) | The Lost City of Yore | None given. | |
| 2 | 1982‑10‑16 (3) | The Magic Fountain | Does not appear. | |
| 2 | 1982‑10‑23 (1) | The Impostor King | Does not appear. | |
| 2 | 1982‑10‑23 (2) | For The Love Of Gargamel | To destroy. | |
| 2 | 1982‑10‑23 (3) | The A-Maze-Ing Smurfs | None given. | Gargamel does say, “This is all your dead end.” |
| 2 | 1982‑10‑23 (4) | The Haunted Castle | Does not appear. | |
| 2 | 1982‑10‑30 (1) | Smurfs At Sea | Does not appear. | |
| 2 | 1982‑10‑30 (2) | One Good Smurf Deserves Another | To eat. | |
| 2 | 1982‑10‑30 (3) | The Blue Plague | To eat. | |
| 2 | 1982‑10‑30 (4) | The Last Laugh | To destroy. | Gargamel later captures some smurfs to use as test subjects. |
| 2 | 1982‑11‑06 (1) | The Raven Wizard | Does not appear. | |
| 2 | 1982‑11‑06 (2) | The Ring of Castellac | Does not appear. | |
| 2 | 1982‑11‑06 (3) | The Sky Is Smurfing, The Sky Is Smurfing | Does not appear. | |
| 2 | 1982‑11‑06 (4) | Turncoat Smurf | None given. | |
| 2 | 1982‑11‑13 (1) | The Return Of Clockwork Smurf | Does not appear. | |
| 2 | 1982‑11‑13 (2) | The Littlest Giant | To destroy. | |
| 2 | 1982‑11‑13 (3) | Bubble, Bubble, Smurf in Trouble | To eat. | |
| 2 | 1982‑11‑13 (4) | Smurf Van Winkle | To eat. | |
| 2 | 1982‑11‑20 (1) | The Prince And The Peewit | Does not appear. | |
| 2 | 1982‑11‑20 (2) | The Enchanted Baby | Does not appear. | |
| 2 | 1982‑11‑20 (3) | Clumsy Smurfs the Future | To eat. | |
| 2 | 1982‑11‑27 (1) | Sleepwalking Smurfs | None given. | |
| 2 | 1982‑11‑27 (2) | Smurf Me No Flowers | Does not appear. | |
| 2 | 1982‑11‑27 (3) | The Good, The Bad, And The Smurfy | Does not appear. | |
| 2 | 1982‑11‑27 (4) | A Mere Truffle | Does not appear. | |
| 2 | 1982‑12‑04 (1) | The Stuff Dreams Are Smurfed Of | None given. | |
| 2 | 1982‑12‑04 (2) | The Box Of Dirty Tricks | To eat. | |
| 2 | 1982‑12‑04 (3) | Papa’s Wedding Day | Does not appear. | |
| 2 | 1982‑12‑04 (4) | All’s Smurf that Ends Smurfy | To eat. | |
| 2 | 1982‑12‑12 (1) | The Smurfs’ Christmas Special | To destroy. | |
| 2 | 1983‑02‑13 (1) | My Smurfy Valentine | To eat. | |
| 3 | 1983‑09‑17 (1) | Once In A Blue Moon | Does not appear. | |
| 3 | 1983‑09‑17 (2) | All Creatures Great and Smurf | None given. | |
| 3 | 1983‑09‑17 (3) | The Smurf Fire Brigade | To destroy. | |
| 3 | 1983‑09‑17 (4) | The Winged Wizard | To impress other wizards. | To show at the Wizards’ Convention. |
| 3 | 1983‑09‑17 (5) | Every Picture Smurfs A Story | Does not appear. | |
| 3 | 1983‑09‑24 (1) | The First Telesmurf | To eat. | |
| 3 | 1983‑09‑24 (2) | Handy’s Kite | To make gold. | |
| 3 | 1983‑09‑24 (3) | The Magic Earrings | Does not seek the smurfs. | Appears but only briefly, Hogatha is the antagonist. |
| 3 | 1983‑09‑24 (4) | The Last Smurfberry | To make gold and to eat. | |
| 3 | 1983‑10‑01 (1) | A Little Smurf Confidence | Does not appear. | |
| 3 | 1983‑10‑01 (2) | Hogatha’s Heart Throb | None given. | |
| 3 | 1983‑10‑01 (3) | Born Rotten | None given. | |
| 3 | 1983‑10‑01 (4) | The Tear Of A Smurf | Does not appear. | |
| 3 | 1983‑10‑01 (5) | The Miracle Smurfer | To eat. | |
| 3 | 1983‑10‑08 (1) | The Smurf Who Would Be King | Does not appear. | |
| 3 | 1983‑10‑08 (2) | How To Smurf A Rainbow | Does not seek the smurfs. | Gargamel is seeking the leprechaun’s gold. |
| 3 | 1983‑10‑08 (3) | Smurfette For A Day | Does not appear. | |
| 3 | 1983‑10‑08 (4) | Peewit Meets Bigmouth | Does not appear. | |
| 3 | 1983‑10‑08 (5) | Lumbering Smurfs | Does not appear. | |
| 3 | 1983‑10‑15 (1) | Handy’s Sweetheart | Does not appear. | |
| 3 | 1983‑10‑15 (2) | Speak For Yourself Farmer Smurf | To make gold. | Gargamel says he will turn the smurfs into gold, rather than using the smurfs to turn base metal into gold. |
| 3 | 1983‑10‑15 (3) | A Hovel Is Not A Home | To make gold. | |
| 3 | 1983‑10‑15 (4) | Forget Me Smurfs | Does not appear. | |
| 3 | 1983‑10‑15 (5) | The Grumpy Gremlin | Does not appear. | |
| 3 | 1983‑10‑22 (1) | Clumsy Luck | Does not appear. | |
| 3 | 1983‑10‑22 (2) | Willpower Smurfs | To eat. | |
| 3 | 1983‑10‑22 (3) | Baby Smurf Is Missing | Does not appear. | |
| 3 | 1983‑10‑22 (4) | The Smurfs’ Time Capsule | Does not appear. | |
| 3 | 1983‑10‑29 (1) | Wedding Bells For Gargamel | To make gold. | |
| 3 | 1983‑10‑29 (2) | To Smurf A Thief | Does not appear. | |
| 3 | 1983‑10‑29 (3) | Greedy And The Porridge Pot | Does not appear. | |
| 3 | 1983‑10‑29 (4) | Harmony Steals The Show | Does not appear. | |
| 3 | 1983‑10‑29 (5) | The Golden Smurf Award | Does not seek the smurfs. | Appears but only briefly, Hogatha is the antagonist. |
| 3 | 1983‑11‑05 (1) | The Moor’s Baby | Does not appear. | |
| 3 | 1983‑11‑05 (2) | Hefty’s Heart | To make gold and to eat. | |
| 3 | 1983‑11‑05 (3) | A Hug For Grouchy | Does not appear. | |
| 3 | 1983‑11‑05 (4) | The Magic Rattle | Does not appear. | |
| 3 | 1983‑11‑05 (5) | All Hallows’ Eve | None given. | Gargamel proposes several ideas but does not settle on one. |
| 3 | 1983‑11‑05 (6) | The Littlest Witch | Does not appear. | |
| 3 | 1983‑11‑12 (1) | April Smurf Day | To eat. | |
| 3 | 1983‑11‑12 (2) | The Magic Stick | Does not appear. | |
| 3 | 1983‑11‑12 (3) | Baby’s First Christmas | To make gold and to eat. | |
| 3 | 1983‑11‑12 (4) | Beauty Is Only Smurf Deep | Does not appear. | |
| 3 | 1983‑11‑12 (5) | Wolf in Peewit’s Clothing | Does not appear. | |
| 3 | 1983‑11‑12 (6) | A Bell For Azrael | None given. | |
| 3 | 1983‑11‑19 (1) | The Chief Record Smurf | To eat. | |
| 3 | 1983‑11‑19 (2) | Smurfing In Sign Language | None given. | |
| 3 | 1983‑11‑19 (3) | Chip Off The Old Smurf | To destroy. | |
| 3 | 1983‑11‑19 (4) | A Gift For Papa’s Day | To eat. | |
| 3 | 1983‑11‑26 (1) | Good Neighbor Smurf | Does not appear. | |
| 3 | 1983‑11‑26 (2) | The Smurfstone Quest | Does not appear. | |
| 3 | 1983‑11‑26 (3) | Hats Off to Smurfs | None given. | |
| 3 | 1983‑11‑26 (4) | The Noble Stag | Does not appear. | |
| 3 | 1983‑11‑26 (5) | Smurfy Acres | To eat. | |
| 3 | 1983‑11‑26 (6) | No Time For Smurfs | Does not appear. | |
| 5 | 1984‑02‑13 (10) | Smurfily Ever After | To eat. | |
| 3 | 1984‑05‑20 (1) | The Smurfic Games | To destroy. | |
| 4 | 1984‑09‑15 (1) | Symbols Of Wisdom | Does not seek the smurfs. | |
| 4 | 1984‑09‑15 (2) | Blue Eyes Returns | To destroy. | |
| 4 | 1984‑09‑15 (3) | The Secret Of The Village Well | To destroy. | |
| 4 | 1984‑09‑15 (4) | Stop And Smurf The Roses | Does not appear. | |
| 4 | 1984‑09‑15 (5) | Gingerbread Smurfs | Does not appear. | |
| 4 | 1984‑09‑15 (6) | Jokey’s Shadow | Does not appear. | |
| 4 | 1984‑09‑22 (1) | Jokey’s Funny Bone | Does not appear. | |
| 4 | 1984‑09‑22 (2) | Tick Tock Smurfs | Does not appear. | |
| 4 | 1984‑09‑22 (3) | The Master Smurf | To eat. | |
| 4 | 1984‑09‑22 (4) | Tailor’s Magic Needle | Does not appear. | |
| 4 | 1984‑09‑22 (5) | The Traveler | Does not appear. | |
| 4 | 1984‑09‑22 (6) | A Pet For Baby Smurf | To eat. | |
| 4 | 1984‑09‑29 (1) | The Incredible Shrinking Wizard | To destroy. | |
| 4 | 1984‑09‑29 (2) | Breakfast At Greedy’s | To eat. | |
| 4 | 1984‑09‑29 (3) | The Secret Of Shadow Swamp | Does not appear. | |
| 4 | 1984‑09‑29 (4) | The Trojan Smurf | To eat. | |
| 4 | 1984‑09‑29 (5) | Smurf The Other Cheek | Does not appear. | |
| 4 | 1984‑10‑06 (1) | A Float Full Of Smurfs | To make gold and to eat. | |
| 4 | 1984‑10‑06 (2) | Smurfette’s Sweet Tooth | To eat. | |
| 4 | 1984‑10‑06 (3) | Smurf On Wood | To make gold and to eat. | |
| 4 | 1984‑10‑06 (4) | The Smurfomatic Smurfolator | To destroy. | |
| 4 | 1984‑10‑06 (5) | Petrified Smurfs | Does not appear. | |
| 4 | 1984‑10‑13 (1) | Papa’s Worrywarts | Does not appear. | |
| 4 | 1984‑10‑13 (2) | Lazy’s Slumber Party | Does not appear. | |
| 4 | 1984‑10‑13 (3) | The Pussywillow Pixies | Does not appear. | |
| 4 | 1984‑10‑13 (4) | The Bignose Dilemma | To eat. | |
| 4 | 1984‑10‑13 (5) | The Smurfbox Derby | To eat. | |
| 4 | 1984‑10‑20 (1) | A Circus For Baby | Does not appear. | |
| 4 | 1984‑10‑20 (2) | Babes In Wartland | Does not appear. | |
| 4 | 1984‑10‑20 (3) | The Smurfwalk Cafe | To eat. | |
| 4 | 1984‑10‑20 (4) | The Smurfiest of Friends | Does not appear. | |
| 4 | 1984‑10‑20 (5) | Never Smurf Off ’Til Tomorrow | Does not appear. | |
| 4 | 1984‑10‑27 (1) | Bigmouth Smurf | To eat. | |
| 4 | 1984‑10‑27 (2) | Baby’s Enchanted Didey | None given. | |
| 4 | 1984‑10‑27 (3) | The Man In The Moon | None given. | |
| 4 | 1984‑10‑27 (4) | Smurfette’s Golden Tresses | Does not appear. | |
| 4 | 1984‑10‑27 (5) | The Whole Smurf And Nothing But The Smurf | To make gold and to eat. | |
| 4 | 1984‑10‑27 (6) | Gargamel’s Giant | To eat. | |
| 4 | 1984‑11‑10 (1) | The Patchwork Bear | Does not appear. | |
| 4 | 1984‑11‑10 (2) | Hefty And The Wheelsmurfer | To eat. | |
| 4 | 1984‑11‑10 (3) | Hopping Cough Smurfs | To eat. | |
| 4 | 1984‑11‑10 (4) | The Little Orange Horse With The Gold Shoes | Does not seek the smurfs. | |
| 4 | 1984‑11‑10 (5) | Monster Smurf | Does not appear. | |
| 4 | 1984‑11‑10 (6) | The Bad Place | Does not appear. | |
| 4 | 1984‑11‑17 (1) | Smurfing For Ghosts | Does not appear. | |
| 4 | 1984‑11‑17 (2) | The Gargoyle Of Quarrel Castle | Does not appear. | |
| 4 | 1984‑11‑17 (3) | Smurfiplication | To make gold and to eat. | |
| 4 | 1984‑11‑17 (4) | Gargamel’s Misfortune | To make gold and to eat. | |
| 5 | 1985‑09‑21 (1) | Stuck On Smurfs | To destroy. | |
| 5 | 1985‑09‑21 (2) | Puppy | None given. | |
| 5 | 1985‑09‑21 (3) | Papa’s Day Off | Does not appear. | |
| 5 | 1985‑09‑21 (4) | The Smurflings | Does not appear. | |
| 5 | 1985‑09‑21 (5) | He Who Smurfs Last | Does not appear. | |
| 5 | 1985‑09‑21 (6) | Baby’s First Word | To make gold and to eat. | |
| 5 | 1985‑09‑28 (1) | The Masked Pie Smurfer | Does not appear. | |
| 5 | 1985‑09‑28 (2) | Sassette | To destroy. | |
| 5 | 1985‑09‑28 (3) | Papa’s Puppy Prescription | To eat. | |
| 5 | 1985‑09‑28 (4) | Poet’s Writer’s Block | Does not appear. | |
| 5 | 1985‑09‑28 (5) | Smurf A Mile In My Shoes | Does not appear. | |
| 5 | 1985‑10‑05 (1) | Dreamy’s Pen Pals | To eat. | |
| 5 | 1985‑10‑05 (2) | Papa’s Flying Bed | To eat. | |
| 5 | 1985‑10‑05 (3) | Mud Wrestling Smurfs | Does not appear. | |
| 5 | 1985‑10‑05 (4) | The Sand Witch | Does not appear. | |
| 5 | 1985‑10‑05 (5) | Kow-Tow, We Won’t Bow | Does not appear. | |
| 5 | 1985‑10‑12 (1) | Bigmouth’s Friend | To make gold. | |
| 5 | 1985‑10‑12 (2) | Wild And Wooly | To eat. | |
| 5 | 1985‑10‑12 (3) | The Dark-Ness Monster | Does not appear. | |
| 5 | 1985‑10‑12 (4) | The Grouchiest Game In Town | Does not seek the smurfs. | Appears only briefly. |
| 5 | 1985‑10‑12 (5) | Queen Smurfette | Does not appear. | |
| 5 | 1985‑10‑19 (1) | Marco Smurf And The Pepper Pirates | Does not appear. | |
| 5 | 1985‑10‑19 (2) | Educating Bigmouth | Does not appear. | |
| 5 | 1985‑10‑19 (3) | Brainy Smurf, Friend To All The Animals | Does not seek the smurfs. | |
| 5 | 1985‑10‑19 (4) | The Comet Is Coming | To eat. | |
| 5 | 1985‑10‑26 (1) | Happy Unhappiness Day To You | To eat. | |
| 5 | 1985‑10‑26 (2) | The Great Slime Crop Failure | Does not appear. | |
| 5 | 1985‑10‑26 (3) | Papa’s Family Album | To eat. | |
| 5 | 1985‑10‑26 (4) | Love Those Smurfs | Does not appear. | |
| 5 | 1985‑10‑26 (5) | Mutiny On The Smurf | Does not appear. | |
| 5 | 1985‑11‑02 (1) | Things That Go Smurf In The Night | To eat. | |
| 5 | 1985‑11‑02 (2) | Alarming Smurfs | To destroy. | |
| 5 | 1985‑11‑02 (3) | Smurfette’s Rose | Does not appear. | |
| 5 | 1985‑11‑02 (4) | The Mr. Smurf Contest | To eat. | |
| 5 | 1985‑11‑02 (5) | Have You Smurfed Your Pet Today? | To eat. | |
| 5 | 1985‑11‑02 (6) | Unsound Smurfs | Does not appear. | |
| 5 | 1985‑11‑09 (1) | All Work And No Smurf | Does not appear. | |
| 5 | 1985‑11‑09 (2) | Gargamel’s Time Trip | To make gold and to eat. | |
| 5 | 1985‑11‑09 (3) | They’re Smurfing Our Song | Does not appear. | |
| 5 | 1985‑11‑09 (4) | Brainy’s Smarty Party | Does not appear. | |
| 6 | 1986‑09‑13 (1) | Smurflings Part I | To eat and to take their treasure. | |
| 6 | 1986‑09‑13 (2) | Smurflings Part II | To take their treasure. | |
| 6 | 1986‑09‑13 (3) | Smurflings Part III | To take their treasure. | |
| 6 | 1986‑09‑13 (4) | Gargamel’s New Job | To make gold and to eat. | |
| 6 | 1986‑09‑20 (1) | Grouchy Makes A Splash | To eat. | |
| 6 | 1986‑09‑20 (2) | No Smurf Is An Island | Does not appear. | |
| 6 | 1986‑09‑20 (3) | Don Smurfo | To eat. | |
| 6 | 1986‑09‑20 (4) | The Prince And The Hopper | Does not appear. | |
| 6 | 1986‑09‑27 (1) | Smurfette’s Gift | Does not appear. | |
| 6 | 1986‑09‑27 (2) | The Most Popular Smurf | To eat. | |
| 6 | 1986‑09‑27 (3) | A Loss Of Smurfs | Does not appear. | |
| 6 | 1986‑09‑27 (4) | The Last Whippoorwill | Does not appear. | |
| 6 | 1986‑09‑27 (5) | The Color Smurfy | To eat. | |
| 6 | 1986‑10‑04 (1) | Lazy’s Nightmare | Does not appear. | |
| 6 | 1986‑10‑04 (2) | All The Smurf’s A Stage | Does not appear. | |
| 6 | 1986‑10‑04 (3) | Smurfs On Wheels | Does not appear. | |
| 6 | 1986‑10‑04 (4) | The Littlest Viking | Does not appear. | |
| 6 | 1986‑10‑11 (1) | Baby’s New Toy | Does not appear. | |
| 6 | 1986‑10‑11 (2) | Bringing Up Bigfeet | To eat. | |
| 6 | 1986‑10‑11 (3) | The Scarlet Croaker | Does not appear. | |
| 6 | 1986‑10‑11 (4) | Calling Dr. Smurf | Does not appear. | |
| 6 | 1986‑10‑11 (5) | Can’t Smurf The Music | Does not appear. | |
| 6 | 1986‑10‑18 (1) | The Royal Drum | Does not appear. | |
| 6 | 1986‑10‑18 (2) | It’s A Puppy’s Life | To eat. | |
| 6 | 1986‑10‑18 (3) | Sweepy Smurf | Does not appear. | |
| 6 | 1986‑10‑18 (4) | Journey To The Center Of The Smurf | Does not appear. | |
| 6 | 1986‑10‑25 (1) | The Tallest Smurf | Does not appear. | |
| 6 | 1986‑10‑25 (2) | Essence of Brainy | To make gold and to eat. | Gargamel wants to drink Brainy’s essence not eat his flesh. |
| 6 | 1986‑10‑25 (3) | Dr. Evil and Mr. Nice | To eat. | |
| 6 | 1986‑10‑25 (4) | The Root Of Evil | Does not appear. | |
| 6 | 1986‑10‑25 (5) | Tattle Tail Smurfs | To eat. | |
| 6 | 1986‑10‑25 (6) | Greedy Goes On Strike | Does not appear. | |
| 6 | 1986‑11‑01 (1) | Future Smurfed | To eat. | |
| 6 | 1986‑11‑01 (2) | Crying Smurfs | To eat. | |
| 6 | 1986‑11‑01 (3) | Gargamel’s Dummy | None given. | |
| 6 | 1986‑11‑01 (4) | Smurf On The Run | To eat. | |
| 6 | 1986‑11‑01 (5) | A Myna Problem | To eat. | |
| 6 | 1986‑11‑01 (6) | The Horn Of Plenty | To eat. | |
| 6 | 1986‑11‑08 (1) | I Smurf To The Trees | To eat. | |
| 6 | 1986‑11‑08 (2) | Clumsy’s Cloud | Does not appear. | |
| 6 | 1986‑11‑08 (3) | Bookworm Smurf | Does not appear. | |
| 6 | 1986‑11‑08 (4) | Farmer’s Genie | Does not appear. | |
| 6 | 1986‑11‑08 (5) | Master Scruple | To eat. | |
| 6 | 1986‑11‑08 (6) | Scruple’s Sweetheart | To eat. | |
| 6 | 1986‑11‑15 (1) | The World According To Smurflings | Does not appear. | |
| 6 | 1986‑11‑15 (2) | The Enchanted Quill | To make gold and to eat. | |
| 6 | 1986‑11‑15 (3) | The Most Unsmurfy Games | Does not appear. | |
| 6 | 1986‑11‑15 (4) | Put Upon Puppy | To eat. | |
| 6 | 1986‑11‑15 (5) | Heart Of Gold | To eat. | |
| 6 | 1986‑11‑15 (6) | The Village Vandal | To eat. | |
| 6 | 1986‑11‑22 (1) | The Gallant Smurf | Does not appear. | |
| 6 | 1986‑11‑22 (2) | Sassette’s Tooth | To eat. | |
| 6 | 1986‑11‑22 (3) | Snappy’s Way | Does not appear. | |
| 6 | 1986‑11‑22 (4) | Fire Fighting Smurfs | To eat. | |
| 6 | 1986‑11‑22 (5) | Handy’s Window-Vision | To eat. | |
| 6 | 1986‑11‑22 (6) | Papa Smurf, Papa Smurf | To impress other wizards. | Two duplicate Gargamels compete to win a smurf-catching contest. |
| 6 | 1986‑11‑29 (1) | Jokey’s Cloak | Does not appear. | |
| 6 | 1986‑11‑29 (2) | Papa’s Last Spell | To eat. | |
| 6 | 1986‑11‑29 (3) | Lure Of The Orb | Does not appear. | |
| 6 | 1986‑11‑29 (4) | Smurfette’s Flowers | Does not appear. | |
| 6 | 1986‑11‑29 (5) | Reckless Smurfs | To eat. | |
| 6 | 1986‑11‑29 (6) | Head Over Hogatha | To make gold and to eat. | |
| 7 | 1987‑09‑19 (1) | Smurf On The Wild Side Part I | To eat. | Gargamel later decides that he doesn’t want to see them, eat them, or turn them into gold; all he wants to do is destroy them. |
| 7 | 1987‑09‑19 (2) | Smurf On The Wild Side Part II | To destroy. | |
| 7 | 1987‑09‑19 (3) | The Smurflings’ Unsmurfy Friend | To eat. | |
| 7 | 1987‑09‑19 (4) | The Smurfstalker | To make gold and to eat. | Gargamel says he’ll turn the smurfs into gold, rather than using them to turn lead into gold. |
| 7 | 1987‑09‑26 (1) | Poltersmurf | Does not appear. | |
| 7 | 1987‑09‑26 (2) | Baby’s Marvelous Toy | To eat. | |
| 7 | 1987‑09‑26 (3) | Sleepless Smurfs | To eat. | |
| 7 | 1987‑09‑26 (4) | Cut-Up Smurfs | To eat. | |
| 7 | 1987‑09‑26 (5) | Gargamel’s Sweetheart | To make gold and to eat. | |
| 7 | 1987‑10‑03 (1) | Wild About Smurfette | Does not appear. | |
| 7 | 1987‑10‑03 (2) | Sing A Song Of Smurflings | Does not appear. | |
| 7 | 1987‑10‑03 (3) | Smurfing For Gold | To make gold and to eat. | |
| 7 | 1987‑10‑03 (4) | Jokey’s Joke Book | To eat. | |
| 7 | 1987‑10‑03 (5) | Poet’s Storybook | Does not appear. | |
| 7 | 1987‑10‑03 (6) | The Fastest Wizard In The World | To make gold. | |
| 7 | 1987‑10‑10 (1) | Dancing Bear | Does not appear. | |
| 7 | 1987‑10‑10 (2) | Gargamel’s Last Will | To eat. | |
| 7 | 1987‑10‑10 (3) | Sassette’s Bewitching Friendship | To eat. | |
| 7 | 1987‑10‑10 (4) | Azrael’s Brain | To eat. | |
| 7 | 1987‑10‑10 (5) | Castaway Smurfs | Does not appear. | |
| 7 | 1987‑10‑10 (6) | Legendary Smurfs | To impress other wizards. | The wizards of the royal library will pay Gargamel gold for proof of the smurfs’ existence. |
| 7 | 1987‑10‑17 (1) | Smurfing The Unicorns | To eat. | |
| 7 | 1987‑10‑17 (2) | Vanity’s Closest Friend | To eat. | |
| 7 | 1987‑10‑17 (3) | Peewit’s Unscrupulous Adventure | Does not appear. | |
| 7 | 1987‑10‑17 (4) | Nobody Smurf | Does not appear. | |
| 7 | 1987‑10‑24 (1) | Scruple And The Great Book Of Spells | To eat. | |
| 7 | 1987‑10‑24 (2) | Bouncing Smurf | To eat. | |
| 7 | 1987‑10‑24 (3) | The Clockwork Smurfette | To eat. | |
| 7 | 1987‑10‑24 (4) | I Was A Brainy Weresmurf | Does not appear. | |
| 6 | 1987‑10‑24 (5) | The Answer Smurf | To eat. | |
| 7 | 1987‑10‑24 (6) | Vanity’s Wild Adventure | To eat. | |
| 7 | 1987‑10‑31 (1) | Soothsayer Smurfette | To make gold and to eat. | |
| 7 | 1987‑10‑31 (2) | Crooner Smurf | Does not appear. | |
| 7 | 1987‑10‑31 (3) | Papa For A Day | Does not appear. | |
| 7 | 1987‑10‑31 (4) | Flighty’s Plight | None given. | |
| 7 | 1987‑10‑31 (5) | To Coin A Smurf | To make gold and to eat. | |
| 7 | 1987‑10‑31 (6) | Smurfette Unmade | To make gold and to eat. | |
| 7 | 1987‑11‑07 (1) | Foul Feather Fiend | To eat. | |
| 7 | 1987‑11‑07 (2) | Sassette’s Hive | Does not appear. | |
| 7 | 1987‑11‑07 (3) | Little Big Smurf | To eat. | |
| 7 | 1987‑11‑07 (4) | Locomotive Smurfs | To eat. | |
| 7 | 1987‑11‑07 (5) | A Long Table for Grandpa | Does not appear. | |
| 7 | 1987‑11‑07 (6) | Where The Wild Smurfs Are | Does not appear. | |
| 7 | 1987‑11‑14 (1) | The Magic Sack Of Mr. Nicholas | To make gold and to eat. | |
| 7 | 1987‑11‑14 (2) | Swapping Smurfs | Does not appear. | |
| 7 | 1987‑11‑14 (3) | Predictable Smurfs | To eat. | Reason inferred by Lazy. |
| 7 | 1987‑11‑14 (4) | Hefty’s Rival | Does not appear. | |
| 7 | 1987‑11‑14 (5) | Snappy’s Puppet | Does not appear. | |
| 7 | 1987‑11‑14 (6) | Prince Smurf | Does not appear. | |
| 7 | 1987‑11‑21 (1) | The Return Of Don Smurfo | None given. | |
| 7 | 1987‑11‑21 (2) | Skyscraper Smurfs | Does not appear. | |
| 7 | 1987‑11‑21 (3) | Bad Luck Smurfs | None given. | |
| 7 | 1987‑11‑21 (4) | Smurfing Out Of Time | Does not appear. | |
| 7 | 1987‑11‑21 (5) | A Hole In Smurf | To eat. | |
| 7 | 1987‑11‑28 (1) | Smurf Pet | Does not appear. | |
| 7 | 1987‑11‑28 (2) | Timber Smurf | To eat. | |
| 7 | 1987‑11‑28 (3) | The Smurf Who Could Do No Wrong | Does not appear. | |
| 7 | 1987‑11‑28 (4) | Smurfette’s Lucky Star | To eat. | |
| 7 | 1987‑11‑28 (5) | The Smurfy Verdict | Does not appear. | |
| 7 | 1987‑11‑28 (6) | Chlorhydris’ Lost Love | Does not appear. | |
| 7 | 1987‑12‑05 (1) | Stop And Go Smurfs | Does not appear. | |
| 7 | 1987‑12‑05 (2) | Poet The Know-It-All | Does not appear. | |
| 7 | 1987‑12‑05 (3) | All The News That’s Fit To Smurf | Does not appear. | |
| 7 | 1987‑12‑05 (4) | Gargamel’s Quest | To make gold. | |
| 7 | 1987‑12‑05 (5) | Gargamel’s Second Childhood | To make gold and to eat. | Gargamel says he will turn the smurfs into gold, rather than using the smurfs to turn base metal into gold. |
| 7 | 1987‑12‑13 (1) | ’Tis the Season To Be Smurfy | Does not appear. | |
| 8 | 1988‑09‑10 (1) | The Lost Smurf | Does not appear. | |
| 8 | 1988‑09‑10 (2) | Archives Of Evil | Does not appear. | |
| 8 | 1988‑09‑17 (1) | Bigmouth’s Roommate | To eat. | |
| 8 | 1988‑09‑17 (2) | Bungling Babysitters | Does not appear. | |
| 8 | 1988‑09‑17 (3) | Clockwork’s Powerplay | To eat. | |
| 8 | 1988‑09‑17 (4) | Clumsy In Command | Does not appear. | |
| 8 | 1988‑09‑24 (1) | Don Smurfo’s Uninvited Guests | To eat. | Book equivalent “Malagarg.” |
| 8 | 1988‑09‑24 (2) | Denisa’s Greedy Doll | To eat. | |
| 8 | 1988‑09‑24 (3) | Denisa’s Slumber Party | To eat. | |
| 8 | 1988‑10‑01 (1) | Grandpa’s Nemesis | To eat. | |
| 8 | 1988‑10‑01 (2) | Grandpa’s Walking Stick | Does not appear. | |
| 8 | 1988‑10‑01 (3) | A House For Nanny | Does not appear. | |
| 8 | 1988‑10‑08 (1) | It’s A Smurfy Life | To eat. | |
| 8 | 1988‑10‑08 (2) | Land Of The Lost And Found | Does not appear. | |
| 8 | 1988‑10‑08 (3) | Long Live Brainy | Does not appear. | |
| 8 | 1988‑10‑15 (1) | A Maze Of Mirrors | Does not appear. | |
| 8 | 1988‑10‑15 (2) | Memory Melons | Does not appear. | |
| 8 | 1988‑10‑15 (3) | Nanny’s Way | To eat. | |
| 8 | 1988‑10‑22 (1) | Pappy’s Puppy | To eat. | |
| 8 | 1988‑10‑22 (2) | Shutterbug Smurfs | To eat. | |
| 8 | 1988‑10‑22 (3) | Smoogle Sings the Blues | Does not appear. | |
| 8 | 1988‑10‑22 (4) | A Smurf For Denisa | To make gold and to eat. | |
| 8 | 1988‑10‑29 (1) | Smurf The Presses | To eat. | |
| 8 | 1988‑10‑29 (2) | Stealing Grandpa’s Thunder | Does not appear. | |
| 9 | 1989‑09‑09 (1) | The Smurfs That Time Forgot | Does not appear. | |
| 9 | 1989‑09‑09 (2) | Lost In The Ages | Does not appear. | |
| 9 | 1989‑09‑09 (3) | Cave Smurfs | Does not appear. | |
| 9 | 1989‑09‑16 (1) | Hogapatra’s Beauty Sleep | Does not appear. | |
| 9 | 1989‑09‑16 (2) | Mummy Dearest | Slave labor and cat food. | Ancient Egypt equivalent “Gargotep.” |
| 9 | 1989‑09‑16 (3) | Shamrock Smurfs | Does not appear. | |
| 9 | 1989‑09‑23 (1) | Karate Clumsy | Does not appear. | |
| 9 | 1989‑09‑23 (2) | Like It Or Smurf It | Does not appear. | |
| 9 | 1989‑09‑23 (3) | Papa’s Big Snooze | Does not appear. | |
| 9 | 1989‑09‑30 (1) | A Fish Called Snappy | Does not appear. | |
| 9 | 1989‑09‑30 (2) | The Smurf Odyssey | Does not appear. | |
| 9 | 1989‑09‑30 (3) | Trojan Smurfs | Does not appear. | |
| 9 | 1989‑10‑07 (1) | Fortune Cookie | Does not appear. | |
| 9 | 1989‑10‑07 (2) | Imperial Panda-Monium | Does not appear. | |
| 9 | 1989‑10‑07 (3) | Smurfette’s Green Thumb | Does not appear. | |
| 9 | 1989‑10‑14 (1) | Hefty Sees A Serpent | As bait for a sea serpent. | Scottish equivalent “MacGarg.” |
| 9 | 1989‑10‑14 (2) | Phantom Bagpiper | Does not appear. | |
| 9 | 1989‑10‑14 (3) | Jungle Jitterbug | Does not appear. | |
| 9 | 1989‑10‑21 (1) | The Clumsy Genie | Does not appear. | |
| 9 | 1989‑10‑21 (2) | Scary Smurfs | Does not appear. | |
| 9 | 1989‑10‑21 (3) | Sky High Surprise | Does not appear. | |
| 9 | 1989‑10‑28 (1) | Gnoman Holiday | Does not appear. | |
| 9 | 1989‑10‑28 (2) | Greedy’s Masterpizza | Does not seek the smurfs. | Ancient Roman equivalent “Gargonzola.” |
| 9 | 1989‑10‑28 (3) | The Monumental Grouch | Does not appear. | |
| 9 | 1989‑11‑04 (1) | Curried Smurfs | To sell for gold. | Indian equivalent “Gargapuri.” |
| 9 | 1989‑11‑04 (2) | G’Day Smoogle | Does not appear. | |
| 9 | 1989‑11‑04 (3) | Grandpa’s Fountain of Youth | Does not appear. | |
| 9 | 1989‑11‑11 (1) | Big Shot Smurfs | Does not appear. | |
| 9 | 1989‑11‑11 (2) | No Reflection On Vanity | Does not appear. | |
| 9 | 1989‑11‑11 (3) | Papa Loses His Patience | Does not seek the smurfs. | Spanish equivalent “El Gargo.” |
| 9 | 1989‑11‑11 (4) | Swashbuckling Smurfs | Does not appear. | |
| 9 | 1989‑11‑18 (1) | Painter’s Egg-Cellent Adventure | Does not seek the smurfs. | Russian equivalent “Gargovitch.” |
| 9 | 1989‑11‑18 (2) | Small-Minded Smurfs | Does not appear. | |
| 9 | 1989‑11‑18 (3) | Bananas Over Hefty | Does not appear. | |
| 9 | 1989‑11‑18 (4) | The Smurfs Of The Round Table | Does not appear. | |
| 9 | 1989‑12‑02 (1) | Wild Goes Cuckoo | Does not appear. | |
| 9 | 1989‑12‑02 (2) | Brainy’s Beastly Boo-Boo | Does not appear. | |
| 9 | 1989‑12‑02 (3) | The Golden Rhino | Does not appear. | |
| 9 | 1989‑12‑02 (4) | Hearts ’N’ Smurfs | Uses Brainy to spread hate. | Holland equivalent “Van Garg.” |